Dynamically reconfigurable electronic and phononic properties in intercalated HfS2

Dynamic reconfigurability of material properties is essential to enabling innovative neuromorphic- and quantum-computing paradigms. The unique structure of van der Waals layers can facilitate a robust mechanism for this desired reconfigurability. Here, we present a highly versatile and effective approach, based on electrochemical intercalation of organometallics, to control the electron and phonon behavior in hafnium disulfide. Computational and...