Tuning the activity and selectivity of electroreduction of CO2 to synthesis gas using bimetallic catalysts
Abstract
The electrochemical carbon dioxide reduction reaction to syngas with controlled CO/H2 ratios has been studied on Pd-based bimetallic hydrides using a combination of in situ characterization and density functional theory calculations. When compared with pure Pd hydride, the bimetallic Pd hydride formation occurs at more negative potentials for Pd-Ag, Pd-Cu, and Pd-Ni. Theoretical calculations show that the choice of the second metal has a more...
Paper Details
Title
Tuning the activity and selectivity of electroreduction of CO2 to synthesis gas using bimetallic catalysts
Published Date
Aug 19, 2019
Journal
Volume
10
Issue
1
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