Mechanisms of Two-Color Laser-Induced Field-Free Molecular Orientation
Abstract
Two mechanisms of two-color (\omega + 2\omega) laser-induced field-free molecular orientation, based on the hyperpolarizability and ionization depletion, are explored and compared. The CO molecule is used as a computational example. While the hyperpolarizability mechanism generates small amounts of orientation at intensities below the ionization threshold, ionization depletion quickly becomes the dominant mechanism as soon as ionizing...
Paper Details
Title
Mechanisms of Two-Color Laser-Induced Field-Free Molecular Orientation
Published Date
Sep 12, 2012
Journal
Volume
109
Issue
11
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